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authorBlaise Thompson <blaise@untzag.com>2018-02-28 19:47:36 -0600
committerBlaise Thompson <blaise@untzag.com>2018-02-28 19:47:36 -0600
commit7b507a18e841f56a534dad25e1a68a17cf6fe280 (patch)
tree4300479ea947a73e5960f6c35bc84876e84c018b /mixed_domain
parent9d89c09dfe49aba4c68b6911600715add419babd (diff)
2018-02-28 19:47
Diffstat (limited to 'mixed_domain')
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diff --git a/mixed_domain/chapter.tex b/mixed_domain/chapter.tex
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--- a/mixed_domain/chapter.tex
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@@ -85,7 +85,7 @@ shift (3PEPS) \cite{EmdeMichelF1998a, DeBoeijWimP1996a, DeBoeijWimP1995a, ChoMin
These methods also include fully-coherent methods involving only coherences such as Stimulated
Raman Spectroscopy (SRS) \cite{YoonSangwoon2005a, McCamantDavidW2005a}, Doubly Vibrationally
Enhanced (DOVE) \cite{ZhaoWei1999a, ZhaoWei1999b, ZhaoWei2000a, MeyerKentA2003a,
- DonaldsonPaulM2007a, DonaldsonPaulM2008a, FournierFrederic2008a},
+ DonaldsonPaulMurray2007b, DonaldsonPaulMurray2008a, FournierFrederic2008a},
Triply Resonant Sum Frequency (TRSF) \cite{BoyleErinSelene2013a, BoyleErinSelene2013b,
BoyleErinSelene2014a}, Sum Frequency Generation (SFG) \cite{LagutchevAlexi2007a}, Coherent
Anti-Stokes Raman Spectroscopy (CARS) \cite{CarlsonRogerJ1990b, CarlsonRogerJ1990c,
@@ -106,13 +106,13 @@ capabilities for measuring homogeneous and inhomogeneous broadening. %
Although these experiments are typically described in the driven
limit, \cite{GallagherSarahM1998a, FourkasJohnT1992a, FourkasJohnT1992b} many of the experiments
involve pulse widths that are comparable to the widths of the system. \cite{MeyerKentA2003a,
- DonaldsonPaulM2007a, PakoulevAndreiV2009a, ZhaoWei1999a, CzechKyleJonathan2015a,
+ DonaldsonPaulMurray2007b, PakoulevAndreiV2009a, ZhaoWei1999a, CzechKyleJonathan2015a,
KohlerDanielDavid2014a} %
MR-CMDS then becomes a mixed-domain experiment whereby resonances are characterized with marginal
resolution in both frequency and time. %
For example, DOVE spectroscopy involves three different pathways \cite{WrightJohnCurtis2003a} whose
relative importance depends on the relative importance of FID and driven
-responses. \cite{DonaldsonPaulM2010a} %
+responses. \cite{DonaldsonPaulMurray2010a} %
In the driven limit, the DOVE line shape depends on the difference between the first two pulse
frequencies so the line shape has a diagonal character that mimics the effects of inhomogeneous
broadening. %
@@ -679,8 +679,8 @@ amplitudes at $t=0$ (driven) and at $t / \Delta_t=2$ (FID); amplitudes for all
$\Omega_{fx}/\Delta_{\omega}$ values shown are comparable at $t=0$, but the lack of FID formation
for $\Omega_{fx}/\Delta_{\omega}=\pm2$ manifests as a visibly disproportionate amplitude decay. %
Many ultrafast spectroscopies take advantage of the latent FID to suppress non-resonant background,
-improving signal to noise. \cite{LagutchevAlexi2007a, LagutchevAlexi2010a, DonaldsonPaulM2010a,
- DonaldsonPaulM2008a} %
+improving signal to noise. \cite{LagutchevAlexi2007a, LagutchevAlexi2010a,
+ DonaldsonPaulMurray2010a, DonaldsonPaulMurray2008a} %
In driven experiments, the output frequency and line shape are fully constrained by the excitation
beams. %
@@ -863,8 +863,8 @@ As a result, the line shape acquires a diagonal character. %
The changes in line shape seen in Fig. \ref{fig:pw1} have significant ramifications for the
interpretations and strategies of MR-CMDS in the mixed domain. %
Time-gating has been used to isolate the 2D spectra of a certain
-time-ordering\cite{MeyerKentA2004a, PakoulevAndreiV2006a, DonaldsonPaulM2007a}, but here we show that
-time-gating itself causes significant line shape changes to the isolated pathways. %
+time-ordering\cite{MeyerKentA2004a, PakoulevAndreiV2006a, DonaldsonPaulMurray2007b}, but here we
+show that time-gating itself causes significant line shape changes to the isolated pathways. %
The phenomenon of time-gating can cause frequency and delay axes to become functional of each other
in unexpected ways. %