2018-04-07 19:02

2 files changed, 45 insertions, 17 deletions

diff --git a/spectroscopy/auto/chapter.el b/spectroscopy/auto/chapter.el
index f8550da..6fd7dd7 100644
--- a/spectroscopy/auto/chapter.el
+++ b/spectroscopy/auto/chapter.el
@@ -3,6 +3,7 @@
  (lambda ()
    (LaTeX-add-labels
     "cha:spc"
-    "spc:fig:decongestion"))
+    "spc:fig:decongestion"
+    "spc:fig:power_curves"))
  :latex)
 
diff --git a/spectroscopy/chapter.tex b/spectroscopy/chapter.tex
index b07a407..eb41d10 100644
--- a/spectroscopy/chapter.tex
+++ b/spectroscopy/chapter.tex
@@ -1,15 +1,3 @@
-% TODO: discuss and cite CerulloGiulio2003.000

-% TODO: discuss and cite BrownEmilyJ1999.000

-% TODO: cite and discuss Sheik-Bahae 1990 (first z-scan)

-% Modeling of Transient Absorption Spectra in Exciton–Charge-Transfer Systems 10.1021/acs.jpcb.6b09858

-% TODO: Multidimensional Spectral Fingerprints of a New Family of Coherent Analytical Spectroscopies

-% TODO: https://www.nature.com/articles/nature21425

-% TODO: https://journals.aps.org/prl/abstract/10.1103/PhysRevLett.76.4793

-% TODO: https://www.nature.com/articles/ncomms2405

-% TODO: https://www.nature.com/articles/ncomms2405

-% TODO: https://pubs.acs.org/doi/abs/10.1021/acs.jpcb.7b02693

-% TODO: http://journals.sagepub.com/doi/10.1177/0003702816669730

-

 \chapter{Spectroscopy} \label{cha:spc}

 

 \begin{dquote}

@@ -144,8 +132,7 @@ WMEL diagrams are drawn using the following rules.  %
 	\item Bra-side interactions are represented with dashed arrows.

 	\item Output is represented as a solid wavy line.

 \end{denumerate}

-

-Representative WMELs can be found in Figures [xxxxxx].  %

+WMELs can be found throughout this dissertation.  %

 

 \section{Types of spectroscopy}  % ================================================================

 

@@ -267,7 +254,7 @@ Besides the aforementioned phase information, probably the biggest difference be
 and homodyne-detected experiments is their scaling with oscillator number density, $N$.  %

 In all heterodyne spectroscopies, signal goes linearly, as $N$.  %

 If the number of oscillators is doubled, the signal doubles.  %

-In all homodyne spectroscopies, signal goes as $N^2$.  %

+In all homodyne spectroscopies, signal goes as $N^2$.  % 

 If the number of oscillators is doubled, the signal goes up by four times.  %

 This is what we mean when we say that homodyne signals are ``intensity level'' and heterodyne

 signals are ``amplitude level''.  %

@@ -292,10 +279,50 @@ In this section I introduce the key components of the MR-CMDS instrument.  %
 

 \subsection{LASER}  % -----------------------------------------------------------------------------

 

-% TODO: add reference to MaimanTheodore.000 (ruby laser)

+Light Amplified by Stimulated Emission of Radiation (LASER) light sources are absolutely crucial

+components of the modern MR-CMDS instrument.  %

+The first laser was built in 1960 by \textcite{MaimanTheodore1960a}, and pulsed lasers were

+invented soon after [CITE].  %

+Today, ultrafast light sources are relatively cheap and reliable.  %

+Our SpectraPhysics ``Tsunami'' oscillator uses passive Kerr-lens mode-locking to generate $\sim$35

+fs seed pulses at $\sim$80 MHz (one pulse every 12.5 nanoseconds). \cite{Tsunami}  %

+This seed is split and fed into two 1 KHz amplifiers, a picosecond ``Spitfire Ace''

+\cite{SpitfireAce} and a femtosecond ``Spitfire Pro'' \cite{SpitfirePro}.  %

+These amplifiers each output several watts of ultrafast pulses at 1 KHz (one pulse per

+millisecond).  %

 

 \subsection{Optical parametric amplifiers}  % -----------------------------------------------------

 

+Optical Parametric Amplifiers (OPAs) are arguably the most crucial component of modern MR-CMDS, as

+they provide the frequency tunable light sources that we require. \cite{CerulloGiulio2003a}  %

+OPAs provide tunability through three-wave sum and difference frequency generation processes.  %

+``Fundamental'' tunability is achieved by splitting the 800 nm photons into two lower energy

+photons, with a splitting ratio determined by motorized optics.  %

+These split photons are called ``signal'' and ``idler'', with signal being the higher energy and

+idler the lower energy photon.  %

+

+% TODO: paragraph about phase matching conditions and polarization

+

+Signal and idler are then either used directly, or amplified through sum or difference frequency

+processes to provide broadband tuneability.  %

+All available optical processes for the TOPAS-C OPAs \cite{TOPAS-C} used on the femtosecond table

+are shown in \autoref{spc:fig:power_curves}.  %

+

+On the picosecond table we have three separate kinds of OPAs, including one TOPAS-800

+\cite{TOPAS-800} and two OPA-800 models that have been modified with precision micro control

+\cite{PMC} servo motors to provide automated tunability.  %

+

+\begin{figure}

+  \caption[TOPAS-C optical processes]{

+    CAPTION TODO.

+  }

+  \label{spc:fig:power_curves}

+\end{figure}

+

 \subsection{Delay stages}  % ----------------------------------------------------------------------

 

+Delay stages are simple, one-motor devices which...

+

 \subsection{Spectrometers}  % ---------------------------------------------------------------------

+

+Spectrometers...
\ No newline at end of file