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author | Blaise Thompson <blaise@untzag.com> | 2018-04-09 00:24:18 -0500 |
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committer | Blaise Thompson <blaise@untzag.com> | 2018-04-09 00:24:18 -0500 |
commit | 357568e1fb77afed9dfa203e62da237bf7ce51b3 (patch) | |
tree | 57b8ddafd412934f1e72b7e1f7fe0256480938fd /PbSe_global_analysis/conclusion.tex | |
parent | e43de3cb79a9fad846babf0ddfdca21622b903dc (diff) |
2018-04-09 00:24
Diffstat (limited to 'PbSe_global_analysis/conclusion.tex')
-rw-r--r-- | PbSe_global_analysis/conclusion.tex | 7 |
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diff --git a/PbSe_global_analysis/conclusion.tex b/PbSe_global_analysis/conclusion.tex new file mode 100644 index 0000000..e7491d1 --- /dev/null +++ b/PbSe_global_analysis/conclusion.tex @@ -0,0 +1,7 @@ +By combining TA and TG measurements, we have described the complex third-order, 2D susceptibility of the 1S resonance of PbSe quantum dots.
+We have demonstrated a parameter extraction procedure that is reproducible for different quantum dot samples, and that some of the parameters, such as the pure dephasing time, are batch dependent.
+Inhomogeneity, exciton-induced broadening, exciton-exciton coulombic coupling shifts, and intraband absorption are all required to reconcile both datasets.
+TA features about 1S exciton band are not exclusively assigned as 1S transitions, which can have important consequences for interpreting the evolution of the 1S bleach.
+
+While the TA spectra show prominent 1S-resonant features, the intraband absorption and its associated refractive index signature are most visible in the TG dataset, so that disentangling the 1S resonant response and the broadband response is a more well-defined problem when both datasets are used together.
+This approach is thus useful for characterization of non-linear signals in spectrally congested systems.
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