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|
@article{Besemann2004,
author = {Besemann, Daniel M. and Meyer, Kent A. and Wright, John C.},
title = {{Spectroscopic Characteristics of Triply Vibrationally
Enhanced Four-Wave Mixing Spectroscopy †}},
journal = {The Journal of Physical Chemistry B},
volume = 108,
number = 29,
pages = {10493--10504},
year = 2004,
doi = {10.1021/jp049597l},
url = {http://pubs.acs.org/doi/abs/10.1021/jp049597l},
abstract = {Triply vibrationally enhanced (TRIVE) four-wave mixing is a
fully resonant, frequency domain spectroscopy that is capable
of coherent multidimensional vibrational spectroscopy. TRIVE
has 12 different coherence pathways that differ in their time
ordering and resonances. The pathways are the coherent
analogue to two-color pump-probe pathways. Specific pathways
or sets of pathways can be chosen by appropriate selection of
time delays and resonance conditions. The pathways have
characteristic positions and line shapes in three-dimensional
frequency space and their coherent interference has
consequences in interpreting the spectra. The line shapes and
the relative intensities of different pathways are dependent
on the population relaxation and dephasing rates. The
different pathways also have different capabilities for
line-narrowing inhomogeneously broadened transitions. The
narrowing is controlled by the interference between pathways
and the quantum level interference between different parts of
the inhomogeneously broadened envelope. We also show that
selection of the output frequency in two-color TRIVE methods
constrains the selection rules that control the relative
transition probabilities of the four transitions.},
file = {::},
issn = {1520-6106},
month = {jul},
}
@article{Block2012,
author = {Block, Stephen B. and Yurs, Lena a. and Pakoulev, Andrei V.
and Selinsky, Rachel Sarah and Jin, Song and Wright, John C.},
title = {{Multiresonant Multidimensional Spectroscopy of
Surface-Trapped Excitons in PbSe Quantum Dots}},
journal = {The Journal of Physical Chemistry Letters},
volume = 3,
number = 18,
pages = {2707--2712},
year = 2012,
doi = {10.1021/jz300599b},
url = {http://pubs.acs.org/doi/abs/10.1021/jz300599b},
file = {::},
issn = {1948-7185},
month = {sep},
}
@article{BritoCruz1988,
author = {{Brito Cruz}, C.H. and Gordon, J.P. and Becker, P.C. and Fork,
R.L. and Shank, C.V.},
title = {{Dynamics of spectral hole burning}},
journal = {IEEE Journal of Quantum Electronics},
volume = 24,
number = 2,
pages = {261--269},
year = 1988,
doi = {10.1109/3.122},
url = {http://ieeexplore.ieee.org/document/122/},
file = {::},
issn = {0018-9197},
month = {feb},
}
@article{Carlson1989,
author = {Carlson, Roger J. and Wright, John C.},
title = {{Absorption and Coherent Interference Effects in Multiply
Resonant Four-Wave Mixing Spectroscopy}},
journal = {Applied Spectroscopy},
volume = 43,
number = 7,
pages = {1195--1208},
year = 1989,
doi = {10.1366/0003702894203408},
url =
{http://openurl.ingenta.com/content/xref?genre=article{\&}issn=0003-7028{\&}volume=43{\&}issue=7{\&}spage=1195},
abstract = {The effects of coherent interference between resonant and
nonresonant signals and the effects of absorption on
multiresonant four-wave mixing spectra are investigated both
theoretically and experimentally in azu- iene-doped
naphthalene crystals at 2 K. Both effects can strongly alter
line shapes and intensities. Line splittings and negative
spectral features are demonstrated. Coherent interference,
although measurable in this system, is weak. Absorption,
however, plays an important role, and its effects on phase
matching, peak shapes, and peak intensities are pre- dicted
theoretically and are confirmed by the experimental measure-
ments. A new expression for the four-wave mixing is derived in
terms of sample absorption coefficients and absorption cross
sections, and gen- eral conditions for maximum efficiency are
determined.},
file = {::},
issn = 00037028,
keywords = {M-factors},
mendeley-tags ={M-factors},
month = {sep},
}
@article{Czech2015,
author = {Czech, Kyle J. and Thompson, Blaise J. and Kain, Schuyler and
Ding, Qi and Shearer, Melinda J. and Hamers, Robert J. and
Jin, Song and Wright, John C.},
title = {{Measurement of Ultrafast Excitonic Dynamics of Few-Layer MoS
2 Using State-Selective Coherent Multidimensional
Spectroscopy}},
journal = {ACS Nano},
volume = 9,
number = 12,
pages = {12146--12157},
year = 2015,
doi = {10.1021/acsnano.5b05198},
url = {http://pubs.acs.org/doi/abs/10.1021/acsnano.5b05198},
abstract = {We report the first coherent multidimensional spectroscopy
study of a MoS2 film. A four-layer sample of MoS2 was
synthesized on a silica substrate by a simplified sulfidation
reaction and characterized by absorption and Raman
spectroscopy, atomic force microscopy, and transmission
electron microscopy. State-selective coherent multidimensional
spectroscopy (CMDS) on the as-prepared MoS2 film resolved the
dynamics of a series of diagonal and cross-peak features
involving the spin-orbit split A and B excitonic states and
continuum states. The spectra are characterized by striped
features that are similar to those observed in CMDS studies of
quantum wells where the continuum states contribute strongly
to the initial excitation of both the diagonal and cross-peak
features, while the A and B excitonic states contributed
strongly to the final output signal. The strong contribution
from the continuum states to the initial excitation shows that
the continuum states are coupled to the A and B excitonic
states and that fast intraband relaxation is occurring on a
sub-70 fs time scale. A comparison of the CMDS excitation
signal and the absorption spectrum shows that the relative
importance of the continuum states is determined primarily by
their absorption strength. Diagonal and cross-peak features
decay with a 680 fs time constant characteristic of exciton
recombination and/or trapping. The short time dynamics are
complicated by coherent and partially coherent pathways that
become important when the excitation pulses are temporally
overlapped. In this region, the coherent dynamics create
diagonal features involving both the excitonic states and
continuum states, while the partially coherent pathways
contribute to cross-peak features.},
file = {::},
issn = {1936-0851},
keywords = {2D,2d,are layered,molybdenum sul fi de,molybdenum
sulfide,multidimensional,nonlinear,ransition metal
dichalcogenides,semiconductors with strong spin,such as mos
2,tmdcs,transition metal dichalcogenides,ultrafast
dynamics,{\`{a}}},
month = {dec},
pmid = 26525496,
}
@article{Dai2009,
author = {Dai, Quanqin and Wang, Yingnan Yiding and Li, Xinbi and Zhang,
Yu and Pellegrino, Donald J. and Zhao, Muxun and Zou, Bo and
Seo, JaeTae and Wang, Yingnan Yiding and Yu, William W.},
title = {{Size-dependent composition and molar extinction coefficient
of PbSe semiconductor nanocrystals.}},
journal = {ACS nano},
volume = 3,
number = 6,
pages = {1518--24},
year = 2009,
doi = {10.1021/nn9001616},
url = {http://www.ncbi.nlm.nih.gov/pubmed/19702314},
abstract = {Atomic compositions and molar extinction coefficients of PbSe
semiconductor nanocrystals were determined by atomic
absorption spectrometry, UV-vis-NIR spectrophotometry, and
transmission electron microscopy. The Pb/Se atomic ratio was
found to be size-dependent with a systematic excess of Pb
atoms in the PbSe nanocrystal system. Experimental results
indicated that the individual PbSe nanocrystal was
nonstoichiometric, consisting of a PbSe core and an extra
layer of Pb atoms. For these nonstoichiometric PbSe
semiconductor nanocrystals, we proposed a new computational
approach to calculate the total number of Pb and Se atoms in
different sized particles. This calculation played a key role
on the accurate determination of the strongly size-dependent
extinction coefficient, which followed a power law with an
exponent of approximately 2.5.},
file = {::},
isbn = {1936-0851},
issn = {1936-086X},
keywords = {Composition,Molar extinction coefficient,PbSe,Semiconductor
nanocrystal,Size dependence,informative,size-exciton
correlation},
mendeley-tags ={informative},
month = {jun},
pmid = 19435305,
}
@article{DeGeyter2012,
author = {{De Geyter}, Bram and Geiregat, Pieter and Gao, Yunan and {Ten
Cate}, Sybren and Houtepen, Arjan J. and Schins, Juleon M. and
{Van Thourhout}, Dries and Siebbeles, Laurens D A and Hens,
Zeger},
title = {{Broadband and picosecond intraband absorption in lead based
colloidal quantum dots}},
journal = {ACS Nano},
number = 7,
pages = {6067--6074},
year = 2012,
doi = {10.1109/ICTON.2012.6254469},
abstract = {Using femtosecond transient absorption spectroscopy we
demonstrate that lead chalcogenide nanocrystals show
considerable, photoinduced absorption (PA) in a broad
wavelength range just below the bandgap. The time-dependent
decay of the PA signal correlates with the recovery of the
band gap absorption, indicating that the same carriers are
involved. Based on this, we assign this PA signal to intraband
absorption, i.e., the excitation of photogenerated carriers
from the bottom of the conduction band or the top of the
valence band to higher energy levels in the conduction and
valence band continuum. We confirm our experiments with
tight-binding calculations. This broadband response in the
commercially interesting near to mid-infrared range is very
relevant for ultra high speed all optical signal processing.
We benchmark the performance with bulk-Si and
Si-nanocrystals.},
file = {::},
isbn = 9781467322270,
issn = 21627339,
keywords = {colloidal nanocrystals,free carrier absorption,intraband
absorption,lead chalcogenide,optical signal
processing,tight-binding,transient absorption spectroscopy},
pmid = 22686663,
}
@article{DelCoso2004,
author = {del Coso, Ra{\'{u}}l and Solis, Javier},
title = {{Relation between nonlinear refractive index and third-order
susceptibility in absorbing media}},
journal = {Journal of the Optical Society of America B},
volume = 21,
number = 3,
pages = 640,
year = 2004,
doi = {10.1364/JOSAB.21.000640},
url = {http://www.opticsinfobase.org/abstract.cfm?URI=JOSAB-21-3-640
https://www.osapublishing.org/abstract.cfm?URI=josab-21-3-640},
abstract = {Expressions relating complex third-order optical
susceptibility ($\chi$(3)=$\chi$R(3)+i$\chi$I(3)) with
nonlinear refractive index (n2) and nonlinear absorption
coefficient ($\beta$) have been formulated that eliminate the
commonly used approximation of a negligible linear absorption
coefficient. The resulting equations do not show the
conventional linear dependence of $\chi$R(3) with n2 and
$\chi$I(3) with $\beta$. Nonlinear refraction and absorption
result instead from the interplay between the real and
imaginary parts of the first- and third-order susceptibilities
of the material. This effect is illustrated in the case of a
metal–dielectric nanocomposite for which n2 and $\beta$ values
were experimentally obtained by Z-scan measurements and for
which the use of the new formulas for $\chi$R(3) and
$\chi$I(3) yield a large correction and a sign reversal for
$\chi$I(3).},
file = {::},
issn = {0740-3224},
month = {mar},
pmid = 220057300022,
}
@article{Gdor2012,
author = {Gdor, Itay and Sachs, Hanan and Roitblat, Avishy and
Strasfeld, David B. and Bawendi, Moungi G. and Ruhman,
Sanford},
title = {{Exploring exciton relaxation and multiexciton generation in
PbSe nanocrystals using hyperspectral near-IR probing.}},
journal = {ACS nano},
volume = 6,
number = 4,
pages = {3269--77},
year = 2012,
doi = {10.1021/nn300184n},
url = {http://www.ncbi.nlm.nih.gov/pubmed/22390473},
abstract = {Hyperspectral femtosecond transient absorption spectroscopy is
employed to record exciton relaxation and recombination in
colloidal lead selenide (PbSe) nanocrystals in unprecedented
detail. Results obtained with different pump wavelengths and
fluences are scrutinized with regard to three issues: (1)
early subpicosecond spectral features due to "hot" excitons
are analyzed in terms of suggested underlying mechanisms; (2)
global kinetic analysis facilitates separation of the
transient difference spectra into single, double, and triple
exciton state contributions, from which individual band
assignments can be tested; and (3) the transient spectra are
screened for signatures of multiexciton generation (MEG) by
comparing experiments with excitation pulses both below and
well above the theoretical threshold for multiplication. For
the latter, a recently devised ultrafast pump-probe
spectroscopic approach is employed. Scaling sample
concentrations and pump pulse intensities inversely with the
extinction coefficient at each excitation wavelength overcomes
ambiguities due to direct multiphoton excitation,
uncertainties of absolute absorption cross sections, and low
signal levels. As observed in a recent application of this
method to InAs core/shell/shell nanodots, no sign of MEG was
detected in this sample up to photon energy 3.7 times the band
gap. Accordingly, numerous reports of efficient MEG in other
samples of PbSe suggest that the efficiency of this process
varies from sample to sample and depends on factors yet to be
determined.},
file = {::},
isbn = {1936-086X (Electronic)$\backslash$r1936-0851 (Linking)},
issn = {1936-086X},
keywords = {SADS,carrier multiplication,ciency in nanocrystals has,exciton
cooling,in accord,led,meg effi-,multiexciton
generation,quantum dots,the apparent enhancement of,ultrafast
spectroscopy},
mendeley-tags ={SADS},
month = {apr},
pmid = 22390473,
}
@article{Gdor2013a,
author = {Gdor, Itay and Yang, Chunfan and Yanover, Diana and Sachs,
Hanan and Lifshitz, Efrat and Ruhman, Sanford},
title = {{Novel Spectral Decay Dynamics of Hot Excitons in PbSe
Nanocrystals: A Tunable Femtosecond Pump–Hyperspectral Probe
Study}},
journal = {The Journal of Physical Chemistry C},
volume = 117,
number = 49,
pages = {26342--26350},
year = 2013,
doi = {10.1021/jp409530z},
url = {http://pubs.acs.org/doi/abs/10.1021/jp409530z},
abstract = {Ultrafast exciton cooling in highly monodisperse PbSe
nanocrystals is followed with tunable pump?hyperspectral
near-IR probe spectroscopy. Unexpected kinetic and spectral
correlations between induced bleach and absorption features
are revealed, which are incompatible with standard models for
excited nanocrystal absorption. Interband optical excitation
immediately generates a sharp bleach feature near the 1Sh1Se
transition which is unchanged during exciton thermalization,
while pumping well above the band edge induces an intense
absorption at frequencies just below the band edge which
decays concurrently with a buildup of renewed absorbance at
the 1Ph1Pe peak during exciton cooling. Transient spectra of
hot single and double excitons are nearly indistinguishable,
arguing against the controversial involvement of Auger cooling
in the rapid dissipation of excess energy in excited PbSe QDs.
Finally, quantitative signal analysis shows no signs of
multiexciton generation up to photon energies four times the
sample band gap. Ultrafast exciton cooling in highly
monodisperse PbSe nanocrystals is followed with tunable
pump?hyperspectral near-IR probe spectroscopy. Unexpected
kinetic and spectral correlations between induced bleach and
absorption features are revealed, which are incompatible with
standard models for excited nanocrystal absorption. Interband
optical excitation immediately generates a sharp bleach
feature near the 1Sh1Se transition which is unchanged during
exciton thermalization, while pumping well above the band edge
induces an intense absorption at frequencies just below the
band edge which decays concurrently with a buildup of renewed
absorbance at the 1Ph1Pe peak during exciton cooling.
Transient spectra of hot single and double excitons are nearly
indistinguishable, arguing against the controversial
involvement of Auger cooling in the rapid dissipation of
excess energy in excited PbSe QDs. Finally, quantitative
signal analysis shows no signs of multiexciton generation up
to photon energies four times the sample band gap.},
file = {::},
isbn = 1557522790,
issn = {1932-7447},
month = {dec},
}
@article{Gdor2015,
author = {Gdor, Itay and Shapiro, Arthur and Yang, Chunfan and Yanover,
Diana and Lifshitz, Efrat and Ruhman, Sanford},
title = {{Three-pulse femtosecond spectroscopy of PbSe nanocrystals: 1S
bleach nonlinearity and sub-band-edge excited-state absorption
assignment}},
journal = {ACS Nano},
volume = 9,
number = 2,
pages = {2138--2147},
year = 2015,
doi = {10.1021/nn5074868},
abstract = {Above band-edge photo-excitation of PbSe nanocrystals induces
strong below band-gap absorption as well as a multi-phased
buildup of bleaching in the 1Se1Sh transition. The amplitudes
and kinetics of these features deviate from expectations based
on bi-exciton shifts and state filling which are the
mechanisms usually evoked to explain them. To clarify these
discrepancies, the same transitions are investigated here by
double-pump probe spectroscopy. Re-exciting in the below
band-gap induced absorption characteristic of hot excitons is
shown to produce additional excitons with high probability. In
addition, pump-probe experiments on a sample saturated with
single relaxed excitons proves that the resulting 1Se1Sh
bleach is not linear with the number of excitons per
nanocrystal. This finding holds for two samples differing
significantly in size, demonstrating its generality. Analysis
of the results suggest that below band edge induced absorption
in hot exciton states is due to excited state absorption and
not to shifted absorption of cold carriers, and that 1Se1Sh
bleach signals are not an accurate counter of sample excitons
when their distribution includes multi-exciton states.},
file = {::},
isbn = {1936-0851},
issn = {1936086X},
keywords = {exciton cooling,multiexciton generation,nanocrystals,quantum
dots,ultrafast spectroscopy},
}
@article{Gdor2015a,
author = {Gdor, Itay and Yanover, Dianna and Yang, Chunfan and Shapiro,
Arthur and Lifshitz, Efrat and Ruhman, Sanford},
title = {{Three Pulse Femtosecond Spectroscopy of PbSe Nano-Crystals ;
1S Bleach Nonlinearity and Sub Band-Edge Excited State
Absorption Assignment Three Pulse Femtosecond Spectroscopy of
PbSe nano-Crystals ; 1S Bleach Nonlinearity and Sub Band-edge
Excited State A}},
journal = {ACS Nano},
pages = {2--5},
year = 2015,
doi = {10.1021/nn5074868},
file = {::},
}
@article{Geiregat2014,
author = {Geiregat, Pieter and Houtepen, Arjan J. and Justo, Yolanda and
Grozema, Ferdinand C. and {Van Thourhout}, Dries and Hens,
Zeger},
title = {{Coulomb Shifts upon Exciton Addition to Photoexcited PbS
Colloidal Quantum Dots}},
journal = {The Journal of Physical Chemistry C},
volume = 118,
number = 38,
pages = {22284--22290},
year = 2014,
doi = {10.1021/jp505530k},
url = {http://pubs.acs.org/doi/abs/10.1021/jp505530k},
abstract = {Using ultrafast hyperspectral transient absorption (TA)
spectroscopy, we determine the biexciton addition energies in
PbS quantum dots (QDs) with different sizes when either a cold
or a hot electron−hole pair is added to a QD already
containing a cooled exciton. The observed dependence of this
so-called biexciton addition energy on the QD diameter and the
exciton energy can be rationalized by interpreting the
addition energies as the result of an imbalance in the Coulomb
interactions between the newly created carriers and the
carriers already present in a QD. The obtained results are
therefore relevant from both a fundamental and practical point
of view. They provide experimental data on Coulomb interaction
between charge carriers in confined semiconductors that can be
compared with theoretical estimates. Moreover, understanding
the way hot−cold biexciton addition energies influence the
transient absorption spectrum adds a new element to the
transient absorption toolbox for the optoelectronic properties
of colloidal QDs. ■ INTRODUCTION Colloidal semiconductor
nanocrystals or quantum dots (QDs) are an increasingly
prominent class of low-dimensional nanomaterials that combine
size-tunable electronic and optical properties with a
suitability for solution-based processing. Starting from
fundamental research and theoretical modeling on their unique
physical properties, QDs are now applied in a variety of
domains such as solar energy harvesting, photo-detection, and
light-emitting diodes or displays. 1−5 These applications
typically rely on the linear optical properties of QDs, i.e.,
light absorption by unexcited QDs and light emission by
radiative recombination in excited QDs. On the other hand,
various studies have shown that the spectral and
time-dependent properties of excited QDs can strongly enhance
the performance of QD-based devices in the above mention
applications or enable QDs to be used in completely different
applications. Quantum dots excited with photons having
energies exceeding twice that of the QD bandgap transition
can, for example, dissipate their excess energy by forming
biexcitons in a process called multiple exciton generation
(MEG) that can considerably enhance the short circuit current
of single junction, QD-based solar cells. 2,6−8 Controlling
the recombination rate of biexcitons by nonradiative Auger
processes allowed for the formation of blinking-free QDs and
facilitated the formation of QD-based lasers. 9,10 Moreover,
it was proven that excited QDs exhibit a broadband and
ultrafast photoinduced absorption related to intraband
transitions of either the excited electron or hole, which
could be used for optical modulation. 11,12},
file = {::;::},
issn = {1932-7447},
month = {sep},
}
@article{Gesuele2012,
author = {Gesuele, F and Sfeir, M Y and Murray, C B and Heinz, T F and
Wong, C W},
title = {{Biexcitonic Effects in Excited Ultrafast Supercontinuum
S{\aa}ectroscopy of Carrier Multiplication and Biexctionic
Effects in Excited States of PbS Quantum Dots}},
journal = {Nano letters},
volume = 12,
pages = 2658,
year = 2012,
file = {::},
keywords = {1,2 the strong spatial,based-materials for third-generation
photovol-,carrier multiplication,confinement of electronic
wave,here is great interest,in the properties
of,multiple-exciton generation,qd,quantum dot,solar
cells,taics,ultrafast spectroscopy},
}
@article{Hogemann1996,
author = {H{\"{o}}gemann, Claudia and Pauchard, Marc and Vauthey, Eric},
title = {{Picosecond transient grating spectroscopy: The nature of the
diffracted spectrum}},
journal = {Review of Scientific Instruments},
volume = 67,
number = 10,
pages = {3449--3453},
year = 1996,
doi = {10.1063/1.1147157},
url = {http://link.aip.org/link/RSINAK/v67/i10/p3449/s1{\&}Agg=doi
http://aip.scitation.org/doi/10.1063/1.1147157},
file = {::},
issn = {0034-6748},
month = {oct},
}
@article{Hutchings1992,
author = {Hutchings, D C and Sheik-Bahae, M and Hagan, D J and {Van
Stryland}, E W},
title = {{Kramers-Kronig relations in nonlinear optics}},
journal = {Optical and Quantum Electronics},
volume = 24,
number = 1,
pages = {1--30},
year = 1992,
doi = {10.1007/BF01234275},
url =
{http://dx.doi.org/10.1007/BF01234275{\%}5Cnhttp://www.springerlink.com/index/10.1007/BF01234275},
abstract = {We review dispersion relations, which relate the real part of
the optical susceptibility (refraction) to the imaginary part
(absorption). We derive and discuss these relations as applied
to nonlinear optical systems. It is shown that in the
nonlinear case, for self-action effects the correct form for
such dispersion relations is nondegenerate, i.e. it is
necessary to use multiple frequency arguments. Nonlinear
dispersion relations have been shown to be very useful as they
usually only require integration over a limited frequency
range (corresponding to frequencies at which the absorption
changes), unlike the conventional linear Kramers-Kr{\"{o}}nig
relation which requires integration over all absorbing
frequencies. Furthermore, calculation of refractive index
changes using dispersion relations is easier than a direct
calculation of the susceptibility, as transition rates (which
give absorption coefficients) are, in general, far easier to
calculate than the expectation value of the optical
polarization. Both resonant (generation of some excitation
that is long lived compared with an optical period) and
nonresonant ‘instantaneous' optical nonlinearities are
discussed, and it is shown that the nonlinear dispersion
relation has a common form and can be understood in terms of
the linear Kramers-Kr{\"{o}}nig relation applied to a new
system consisting of the material plus some ‘perturbation'. We
present several examples of the form of this external
perturbation, which can be viewed as the pump in a pump-probe
experiment. We discuss the two-level saturated atom model and
bandfilling in semiconductors among others for the resonant
case. For the nonresonant case some recent work is included
where the electronic nonlinear refractive coefficient,n2, is
determined from the nonlinear absorption processes of
two-photon absorption, Raman transitions and the a.c. Stark
effect. We also review how the dispersion relations can be
extended to give alternative forms for frequency summation
which, for example, allows the real and imaginary parts of?(2)
to be related.},
file = {::;::},
isbn = {0306-8919},
issn = 03068919,
}
@article{Kang1997,
author = {Kang, Inuk and Wise, Frank W.},
title = {{Electronic structure and optical properties of PbS and PbSe
quantum dots}},
journal = {Journal of the Optical Society of America B},
volume = 14,
number = 7,
pages = 1632,
year = 1997,
doi = {10.1364/JOSAB.14.001632},
url =
{http://www.opticsinfobase.org/abstract.cfm?URI=josab-14-7-1632},
file = {:C$\backslash$:/Users/Dan/AppData/Local/Mendeley Ltd./Mendeley
Desktop/Downloaded/Kang, Wise - 1997 - Electronic structure
and optical properties of PbS and PbSe quantum dots.pdf:pdf},
issn = {0740-3224},
month = {jul},
}
@article{Karki2013,
author = {Karki, Khadga J and Ma, Fei and Zheng, Kaibo and Zidek, Karel
and Mousa, Abdelrazek and Abdellah, Mohamed and Messing, Maria
E and Wallenberg, L Reine and Yartsev, Arkadi and Pullerits,
T{\~{o}}nu},
title = {{Multiple exciton generation in nano-crystals revisited:
consistent calculation of the yield based on pump-probe
spectroscopy.}},
journal = {Scientific reports},
volume = 3,
pages = 2287,
year = 2013,
doi = {10.1038/srep02287},
url =
{http://www.pubmedcentral.nih.gov/articlerender.fcgi?artid=3724175{\&}tool=pmcentrez{\&}rendertype=abstract},
abstract = {Multiple exciton generation (MEG) is a process in which more
than one exciton is generated upon the absorption of a high
energy photon, typically higher than two times the band gap,
in semiconductor nanocrystals. It can be observed
experimentally using time resolved spectroscopy such as the
transient absorption measurements. Quantification of the MEG
yield is usually done by assuming that the bi-exciton signal
is twice the signal from a single exciton. Herein we show that
this assumption is not always justified and may lead to
significant errors in the estimated MEG yields. We develop a
methodology to determine proper scaling factors to the signals
from the transient absorption experiments. Using the
methodology we find modest MEG yields in lead chalcogenide
nanocrystals including the nanorods.},
file = {::},
issn = {2045-2322},
month = {jan},
pmid = 23887181,
}
@article{Kohler2014,
author = {Kohler, Daniel D. and Block, Stephen B. and Kain, Schuyler and
Pakoulev, Andrei V. and Wright, John C.},
title = {{Ultrafast Dynamics within the 1S Exciton Band of Colloidal
PbSe Quantum Dots Using Multiresonant Coherent
Multidimensional Spectroscopy}},
journal = {The Journal of Physical Chemistry C},
volume = 118,
number = 9,
pages = {5020--5031},
year = 2014,
doi = {10.1021/jp412058u},
url = {http://pubs.acs.org/doi/abs/10.1021/jp412058u},
file = {::},
issn = {1932-7447},
month = {mar},
}
@article{Kohler2017,
author = {Kohler, Daniel D and Thompson, Blaise J and Wright, John C},
title = {{Frequency-domain coherent multidimensional spectroscopy when
dephasing rivals pulsewidth: Disentangling material and
instrument response}},
journal = {The Journal of Chemical Physics},
volume = 147,
number = 8,
pages = 084202,
year = 2017,
doi = {10.1063/1.4986069},
url = {http://dx.doi.org/10.1063/1.4986069
http://aip.scitation.org/toc/jcp/147/8
http://aip.scitation.org/doi/10.1063/1.4986069},
abstract = {Ultrafast spectroscopy is often collected in the mixed
frequency/time domain, where pulse durations are similar to
system dephasing times. In these experiments, expectations
derived from the familiar driven and impulsive limits are not
valid. This work simulates the mixed-domain four-wave mixing
response of a model system to develop expectations for this
more complex field-matter interaction. We explore frequency
and delay axes. We show that these line shapes are exquisitely
sensitive to excitation pulse widths and delays. Near pulse
overlap, the excitation pulses induce correlations that
resemble signatures of dynamic inhomogeneity. We describe
these line shapes using an intuitive picture that connects to
familiar field-matter expressions. We develop strategies for
distinguishing pulse-induced correlations from true system
inhomogeneity. These simulations provide a founda-tion for
interpretation of ultrafast experiments in the mixed domain.},
file = {::},
issn = {0021-9606},
month = {aug},
}
@article{Kraatz2014,
author = {Kraatz, Ingvar T and Booth, Matthew and Whitaker, Benjamin J
and Nix, Michael G D and Critchley, Kevin},
title = {{Sub-Bandgap Emission and Intraband Defect-Related
Excited-State Dynamics in Colloidal CuInS 2 /ZnS Quantum Dots
Revealed by Femtosecond Pump − Dump − Probe Spectroscopy}},
year = {2014},
file = {::},
}
@article{Lucarini2008,
author = {Lucarini, Valerio},
title = {{Response theory for equilibrium and non-equilibrium
statistical mechanics: Causality and generalized
kramers-kronig relations}},
journal = {Journal of Statistical Physics},
volume = 131,
number = 3,
pages = {543--558},
year = 2008,
doi = {10.1007/s10955-008-9498-y},
abstract = {We consider the general response theory proposed by Ruelle for
describing the impact of small perturbations to the
non-equilibrium steady states resulting from Axiom A dynamical
systems. We show that the causality of the response functions
allows for writing a set of Kramers-Kronig relations for the
corresponding susceptibilities at all orders of nonlinearity.
Nonetheless, only a special class of observable
susceptibilities obey Kramers-Kronig relations. Specific
results are provided for arbitrary order harmonic response,
which allows for a very comprehensive Kramers-Kronig analysis
and the establishment of sum rules connecting the asymptotic
behavior of the susceptibility to the short-time response of
the system. These results generalize previous findings on
optical Hamiltonian systems and simple mechanical models, and
shed light on the general impact of considering the principle
of causality for testing self-consistency: the described
dispersion relations constitute unavoidable benchmarks for any
experimental and model generated dataset. In order to connect
the response theory for equilibrium and non equilibrium
systems, we rewrite the classical results by Kubo so that
response functions formally identical to those proposed by
Ruelle, apart from the measure involved in the phase space
integration, are obtained. We briefly discuss how these
results, taking into account the chaotic hypothesis, might be
relevant for climate research. In particular, whereas the
fluctuation-dissipation theorem does not work for
non-equilibrium systems, because of the non-equivalence
between internal and external fluctuations, Kramers-Kronig
relations might be more robust tools for the definition of a
self-consistent theory of climate change.},
archivePrefix ={arXiv},
arxivId = {0710.0958},
eprint = {0710.0958},
file = {::},
issn = 00224715,
keywords = {Axiom A dynamical systems,Chaotic hypothesis,Climate,Harmonic
generation,Kramers-Kronig relations,Kubo response
theory,Non-equilibrium steady states,Ruelle response
theory,SRB measure},
}
@article{Moreels2006,
author = {Moreels, I. and Hens, Z. and Kockaert, P. and Loicq, J. and
{Van Thourhout}, D.},
title = {{Spectroscopy of the nonlinear refractive index of colloidal
PbSe nanocrystals}},
journal = {Applied Physics Letters},
volume = 89,
number = 19,
pages = {0--4},
year = 2006,
doi = {10.1063/1.2385658},
abstract = {A spectroscopic study of the optical nonlinearity of PbSe
colloidal solutions was performed with the Z-scan technique at
wavelength intervals of 1200-1350 and 1540-1750 nm. While
nonlinear absorption remains below the detection threshold,
the third order nonlinear refractive index n(2) shows clear
resonances, somewhat blueshifted relative to the exciton
transitions in the absorbance spectrum. The occurrence of
thermal effects is ruled out by time-resolved measurements. At
1.55 mu m, measured (resonant) n(2) values exceed typical bulk
semiconductor values by two orders of magnitude. At high
optical intensity, the refractive index change saturates,
indicating that statefilling lies at the origin of the
observed effect.},
file = {::},
isbn = {0003-6951},
issn = 00036951,
}
@article{Moreels2007,
author = {Moreels, Iwan and Lambert, Karel and {De Muynck}, David and
Vanhaecke, Frank and Poelman, Dirk and Martins, Jos{\'{e}} C.
and Allan, Guy and Hens, Zeger},
title = {{Composition and Size-Dependent Extinction Coefficient of
Colloidal PbSe Quantum Dots}},
journal = {Chemistry of Materials},
volume = 19,
number = 25,
pages = {6101--6106},
year = 2007,
doi = {10.1021/cm071410q},
url = {http://pubs.acs.org/doi/abs/10.1021/cm071410q},
file = {::},
issn = {0897-4756},
keywords = {reference,size-exciton correlation},
mendeley-tags ={reference},
month = {dec},
}
@article{Moreels2008,
author = {Moreels, Iwan and Hens, Zeger},
title = {{On the interpretation of colloidal quantum-dot absorption
spectra.}},
journal = {Small (Weinheim an der Bergstrasse, Germany)},
volume = 4,
number = 11,
pages = {1866--8; author reply 1869--70},
year = 2008,
doi = {10.1002/smll.200800068},
url = {http://www.ncbi.nlm.nih.gov/pubmed/18855972},
file = {::},
issn = {1613-6829},
keywords = {Absorption,Colloids,Colloids: chemistry,Quantum Dots,Spectrum
Analysis,Spectrum Analysis: methods},
month = {nov},
pmid = 18855972,
}
@article{Moreels2009,
author = {Moreels, Iwan and Lambert, Karel and Muynck, David De and
Vanhaecke, Frank and Poelman, Dirk and Martins, Jos{\'{e}} C
and Allan, Guy and Hens, Zeger},
title = {{Size-Dependent Optical Properties of Colloidal {\{}PbS{\}}
Quantum Dots}},
journal = {ACS Nano},
volume = 3,
number = 10,
pages = {3023--3030},
year = 2009,
doi = {10.1021/nn900863a},
abstract = {We quantitatively investigate the size-dependent optical
properties of colloidal {\{}PbS{\}} nanocrystals or quantum
dots (Qdots), by combining the Qdot absorbance spectra with
detailed elemental analysis of the Qdot suspensions. At high
energies, the molar extinction coefficient ?? increases with
the Qdot volume d3 and agrees with theoretical calculations
using the Maxwell???Garnett effective medium theory and bulk
values for the Qdot dielectric function. This demonstrates
that quantum confinement has no influence on ?? in this
spectral range, and it provides an accurate method to
calculate the Qdot concentration. Around the band gap, ?? only
increases with d1.3, and values are comparable to the ?? of
{\{}PbSe{\}} Qdots. The data are related to the oscillator
strength fif of the band gap transition and results agree well
with theoretical tight-binding calculations, predicting a
linear dependence of fif on d. For both {\{}PbS{\}} and
{\{}PbSe{\}} Qdots, the exciton lifetime ?? is calculated from
fif. We find values ranging between 1 and 3 ??s, in agreement
with experimental literature data from time-resolved
luminescence spectroscopy. Our results provide a thorough
general framework to calculate and understand the optical
properties of suspended colloidal quantum dots. Most
importantly, it highlights the significance of the local field
factor in these systems.},
file = {::},
issn = {1936-0851},
keywords = {exciton lifetime,extinction coefficient,lead
chalcogenide,molar,oscillator strength,pbse,semiconductor
nanocrystals},
}
@article{Nootz2011,
author = {Nootz, Gero and Padilha, Lazaro A. and Levina, Larissa and
Sukhovatkin, Vlad and Webster, Scott and Brzozowski, Lukasz
and Sargent, Edward H. and Hagan, David J. and {Van Stryland},
Eric W.},
title = {{Size dependence of carrier dynamics and carrier
multiplication in PbS quantum dots}},
journal = {Physical Review B - Condensed Matter and Materials Physics},
volume = 83,
number = 15,
pages = {1--7},
year = 2011,
doi = {10.1103/PhysRevB.83.155302},
abstract = {The time dynamics of the photoexcited carriers and
carrier-multiplication efficiencies in PbS quantum dots (QDs)
are investigated. In particular, we report on the carrier
dynamics, including carrier multiplication, as a function of
QD size and compare them to the bulk value. We show that the
intraband 1P -{\textgreater} 1S decay becomes faster for
smaller QDs, in agreement with the absence of a phonon
bottleneck. Furthermore, as the size of the QDs decreases, the
energy threshold for carrier multiplication shifts from the
bulk value to higher energies. However, the energy threshold
shift is smaller than the band-gap shift and, therefore, for
the smallest QDs, the threshold approaches 2.35 E(g), which is
close to the theoretical energy conservation limit of twice
the band gap. We also show that the carrier-multiplication
energy efficiency increases with decreasing QD size. By
comparing to theoretical models, our results suggest that
impact ionization is sufficient to explain carrier
multiplication in QDs.},
file = {::},
isbn = {1098-0121},
issn = 10980121,
}
@article{Okumura1999,
author = {Okumura, Ko and Tokmakoff, Andrei and Tanimura, Yoshitaka},
title = {{Two-dimensional line-shape analysis of photon-echo signal}},
journal = {Chemical Physics Letters},
volume = 314,
number = {5-6},
pages = {488--495},
year = 1999,
doi = {10.1016/S0009-2614(99)01173-2},
url = {http://linkinghub.elsevier.com/retrieve/pii/S0009261499011732},
abstract = {We analyze the two-dimensional (2D) line shape obtained by 2D
Fourier transforming the time-domain response of a photon-echo
signal as a function of the two coherence periods, t(1) and
t(3). The line shape obtained for a two-level system with
homogeneous and inhomogeneous broadening is shown to be
sensitive to the magnitude of both of these line-broadening
mechanisms. It is shown that the ellipticity of the 2D line
shape can be related to the ratio of homogeneous to
inhomogeneous broadening. (C) 1999 Elsevier Science B.V. All
rights reserved.},
file = {:C$\backslash$:/Users/Dan/AppData/Local/Mendeley Ltd./Mendeley
Desktop/Downloaded/Okumura, Tokmakoff, Tanimura - 1999 -
Two-dimensional line-shape analysis of photon-echo
signal.pdf:pdf},
isbn = {0009-2614},
issn = 00092614,
keywords = {3rd-order,dynamics,glasses,phase,probes,spectroscopy},
month = {dec},
}
@article{Olivero1977,
author = {Olivero, J.J. and Longbothum, R.L.},
title = {{Empirical fits to the voigt line width: A brief review}},
journal = {J. Quant. Spectrosc. Radiat. Transfer},
volume = 17,
pages = {233--236},
year = 1977,
file = {::},
}
@article{Omari2012,
author = {Omari, Abdoulghafar and Moreels, Iwan and Masia, Francesco and
Langbein, Wolfgang and Borri, Paola and {Van Thourhout}, Dries
and Kockaert, Pascal and Hens, Zeger},
title = {{Role of interband and photoinduced absorption in the
nonlinear refraction and absorption of resonantly excited PbS
quantum dots around 1550 nm}},
journal = {Physical Review B},
volume = 85,
number = 11,
pages = 115318,
year = 2012,
doi = {10.1103/PhysRevB.85.115318},
url = {http://link.aps.org/doi/10.1103/PhysRevB.85.115318},
file = {::},
issn = {1098-0121},
month = {mar},
}
@article{Pang1991,
author = {Pang, Yang and Samoc, Marek and Prasad, Paras N.},
title = {{Third‐order nonlinearity and two‐photon‐induced molecular
dynamics: Femtosecond time‐resolved transient absorption, Kerr
gate, and degenerate four‐wave mixing studies in poly ( p
‐phenylene vinylene)/sol‐gel silica film}},
journal = {The Journal of Chemical Physics},
volume = 94,
number = 8,
pages = {5282--5290},
year = 1991,
doi = {10.1063/1.460512},
url =
{http://scitation.aip.org/content/aip/journal/jcp/94/8/10.1063/1.460512
http://aip.scitation.org/doi/10.1063/1.460512},
abstract = {Femtosecond response and relaxation of the third-order optical
nonlinearity in a newly developed poly (p-phenylene
vinylene)/sol-gel silica composite are investigated by time-
resolved forward wave degenerate four-wave mixing, Kerr gate,
and transient absorption techniques using 60 fs pulses at 620
nm. Using a theoretical description of two- and four-wave
mixing in optically nonlinear media, it is shown that the
results obtained from simultaneous use of these techniques
yield valuable information on the real and imaginary
components of the third-order susceptibility. In the composite
material investigated here, the imaginary component is derived
from the presence of a two-photon resonance at the wavelength
of 620 nm used for the present study. This two-photon
resonance is observed as transient absorption of the probe
beam induced by the presence of a strong pump beam. It also
provides fifth-order nonlinear response both in transient
absorption and in degenerate four-wave mixing. The fifth-
order contributions are derived from the two-photon generated
excited species which can absorb at the measurement wavelength
and therefore modify both the absorption coefficient and the
refractive index of the medium.},
file = {::},
issn = {0021-9606},
month = {apr},
}
@article{Peterson2007,
author = {Peterson, JJ and Huang, Libai and Delerue, C. and Allan, Guy},
title = {{Uncovering forbidden optical transitions in PbSe
nanocrystals}},
journal = {nano Letters},
year = 2007,
url = {http://pubs.acs.org/doi/abs/10.1021/nl072487g},
file = {:C$\backslash$:/Users/Dan/AppData/Local/Mendeley Ltd./Mendeley
Desktop/Downloaded/Peterson et al. - 2007 - Uncovering
forbidden optical transitions in PbSe nanocrystals.pdf:pdf},
keywords = {1P exciton,2 photon absorption,new,relevant},
mendeley-tags ={new,relevant},
}
@article{Price2015,
author = {Price, Michael B. and Butkus, Justinas and Jellicoe, Tom C.
and Sadhanala, Aditya and Briane, Anouk and Halpert, Jonathan
E. and Broch, Katharina and Hodgkiss, Justin M. and Friend,
Richard H. and Deschler, Felix},
title = {{Hot-carrier cooling and photoinduced refractive index changes
in organic–inorganic lead halide perovskites}},
journal = {Nature Communications},
volume = 6,
number = {May},
pages = 8420,
year = 2015,
doi = {10.1038/ncomms9420},
url = {http://dx.doi.org/10.1038/ncomms9420
http://www.nature.com/doifinder/10.1038/ncomms9420},
archivePrefix ={arXiv},
arxivId = {arXiv:1504.07508},
eprint = {arXiv:1504.07508},
file = {::},
issn = {2041-1723},
publisher = {Nature Publishing Group},
}
@article{Schaller2003,
author = {Schaller, Richard D and Petruska, M. a. and Klimov, Victor I.},
title = {{Tunable Near-Infrared Optical Gain and Amplified Spontaneous
Emission Using PbSe Nanocrystals}},
journal = {The Journal of Physical Chemistry B},
volume = 107,
number = 50,
pages = {13765--13768},
year = 2003,
doi = {10.1021/jp0311660},
url = {http://pubs.acs.org/doi/abs/10.1021/jp0311660},
file = {::;::},
issn = {1520-6106},
month = {dec},
}
@article{Schins2009,
author = {Schins, Juleon and Trinh, M. and Houtepen, Arjan and
Siebbeles, Laurens},
title = {{Probing formally forbidden optical transitions in PbSe
nanocrystals by time- and energy-resolved transient absorption
spectroscopy}},
journal = {Physical Review B},
volume = 80,
number = 3,
pages = 035323,
year = 2009,
doi = {10.1103/PhysRevB.80.035323},
url = {http://link.aps.org/doi/10.1103/PhysRevB.80.035323},
file = {::},
issn = {1098-0121},
month = {jul},
}
@article{Svirko1999,
author = {{P. Svirko}, Yuri and Shirane, Masayuki and Suzuura, Hidekatsu
and Kuwata-Gonokami, Makoto},
title = {{Four-Wave Mixing Theory at the Excitonic Resonance: Weakly
Interacting Boson Model}},
journal = {Journal of the Physical Society of Japan},
volume = 68,
number = 2,
pages = {674--682},
year = 1999,
doi = {10.1143/JPSJ.68.674},
url = {http://journals.jps.jp/doi/10.1143/JPSJ.68.674},
file = {::},
issn = {0031-9015},
keywords = {Exciton,Four-particle correlation,Four-wave mixing,Normal mode
splitting,Semiconductor microcavity},
month = {feb},
}
@article{Trinh2008,
author = {Trinh, M Tuan and Houtepen, Arjan J and Schins, Juleon M and
Piris, Jorge and Siebbeles, Laurens D a},
title = {{Nature of the second optical transition in PbSe
nanocrystals.}},
journal = {Nano letters},
volume = 8,
number = 7,
pages = {2112--7},
year = 2008,
doi = {10.1021/nl8010963},
url = {http://www.ncbi.nlm.nih.gov/pubmed/18510369},
abstract = {The second peak in the optical absorption spectrum of PbSe
nanocrystals is arguably the most discussed optical transition
in semiconductor nanocrystals. Ten years of scientific debate
have produced many theoretical and experimental claims for the
assignment of this feature as the 1P e1P h as well as the 1S
h,e1P e,h transitions. We studied the nature of this
absorption feature by pump-probe spectroscopy, exactly
controlling the occupation of the states involved, and present
conclusive evidence that the optical transition involves
neither 1S e nor 1S h states. This suggests that it is the 1P
h1P e transition that gives rise to the second peak in the
absorption spectrum of PbSe nanocrystals.},
file = {::},
issn = {1530-6984},
month = {jul},
pmid = 18510369,
}
@article{Trinh2013,
author = {Trinh, M. Tuan and Sfeir, Matthew Y. and Choi, Joshua J. and
Owen, Jonathan S. and Zhu, Xiaoyang},
title = {{A Hot Electron–Hole Pair Breaks the Symmetry of a
Semiconductor Quantum Dot}},
journal = {Nano Letters},
volume = 13,
number = 12,
pages = {6091--6097},
year = 2013,
doi = {10.1021/nl403368y},
url = {http://pubs.acs.org/doi/abs/10.1021/nl403368y},
file = {::},
issn = {1530-6984},
keywords = {google the phrase,hot carriers,nanocrystals or,near the
bandgap is,now well-,one,ptical excitation of
semiconductor,qds,quantum dots,selection rules,stark
effect,symmetry breaking,transient absorption,understood},
month = {dec},
}
@article{Wehrenberg2002,
author = {Wehrenberg, Brian L. and Wang, Congjun and Guyot-Sionnest,
Philippe},
title = {{Interband and Intraband Optical Studies of PbSe Colloidal
Quantum Dots}},
journal = {The Journal of Physical Chemistry B},
volume = 106,
number = 41,
pages = {10634--10640},
year = 2002,
doi = {10.1021/jp021187e},
url = {http://pubs.acs.org/doi/abs/10.1021/jp021187e},
file = {::},
issn = {1520-6106},
month = {oct},
}
@article{Wise2000,
author = {Wise, Frank W.},
title = {{Lead salt quantum dots: the limit of strong quantum
confinement.}},
journal = {Accounts of chemical research},
volume = 33,
number = 11,
pages = {773--80},
year = 2000,
url = {http://www.ncbi.nlm.nih.gov/pubmed/11087314},
abstract = {Nanocrystals or quantum dots of the IV-VI semiconductors PbS,
PbSe, and PbTe provide unique properties for investigating the
effects of strong confinement on electrons and phonons. The
degree of confinement of charge carriers can be many times
stronger than in most II-VI and III-V semiconductors, and lead
salt nanostructures may be the only materials in which the
electronic energies are determined primarily by quantum
confinement. This Account briefly reviews recent research on
lead salt quantum dots.},
file = {:C$\backslash$:/Users/Dan/AppData/Local/Mendeley Ltd./Mendeley
Desktop/Downloaded/Wise - 2000 - Lead salt quantum dots the
limit of strong quantum confinement.pdf:pdf},
issn = {0001-4842},
keywords = {Crystallization,Electrochemistry,Lead,Lead:
chemistry,Semiconductors,Temperature},
month = {nov},
pmid = 11087314,
}
@article{Yang2015,
author = {Yang, Ye and Yan, Yong and Yang, Mengjin and Choi, Sukgeun and
Zhu, Kai and Luther, Joseph M and Beard, Matthew C},
title = {{Low surface recombination velocity in}},
journal = {Nature Communications},
volume = 6,
pages = {1--6},
year = 2015,
doi = {10.1038/ncomms8961},
url = {http://dx.doi.org/10.1038/ncomms8961},
file = {::},
publisher = {Nature Publishing Group},
}
@article{Yang2017,
author = {Yang, Ye and Yang, Mengjin and Moore, David?T. and Yan, Yong
and Miller, Elisa?M. and Zhu, Kai and Beard, Matthew?C.},
title = {{Top and bottom surfaces limit carrier lifetime in lead iodide
perovskite films}},
journal = {Nature Energy},
volume = 2,
number = 2,
pages = 16207,
year = 2017,
doi = {10.1038/nenergy.2016.207},
url = {http://www.nature.com/articles/nenergy2016207},
abstract = {Carrier recombination at defects is detrimental to the
performance of solar energy conversion systems, including
solar cells and photoelectrochemical devices. Point defects
are localized within the bulk crystal while extended defects
occur at surfaces and grain boundaries. If not properly
managed, surfaces can be a large source of carrier
recombination. Separating surface carrier dynamics from bulk
and/or grain-boundary recombination in thin films is
challenging. Here, we employ transient reflection spectroscopy
to measure the surface carrier dynamics in methylammonium lead
iodide perovskite polycrystalline films. We find that surface
recombination limits the total carrier lifetime in perovskite
polycrystalline thin films, meaning that recombination inside
grains and/or at grain boundaries is less important than top
and bottom surface recombination. The surface recombination
velocity in polycrystalline films is nearly an order of
magnitude smaller than that in single crystals, possibly due
to unintended surface passivation of the films during
synthesis.},
file = {::},
issn = {2058-7546},
month = {jan},
}
@article{Yurs2011,
author = {Yurs, Lena A and Block, Stephen B and Pakoulev, Andrei V. and
Selinsky, Rachel S. and Jin, Song and Wright, John},
title = {{Multiresonant Coherent Multidimensional Electronic
Spectroscopy of Colloidal PbSe Quantum Dots}},
journal = {The Journal of Physical Chemistry C},
volume = 115,
number = 46,
pages = {22833--22844},
year = 2011,
doi = {10.1021/jp207273x},
url = {http://pubs.acs.org/doi/abs/10.1021/jp207273x},
file = {::},
issn = {1932-7447},
month = {nov},
}
@article{Yurs2012,
author = {Yurs, Lena A and Block, Stephen B and Pakoulev, Andrei V. and
Selinsky, Rachel S. and Jin, Song and Wright, John},
title = {{Spectral Isolation and Measurement of Surface-Trapped State
Multidimensional Nonlinear Susceptibility in Colloidal Quantum
Dots}},
journal = {The Journal of Physical Chemistry C},
volume = 116,
number = 9,
pages = {5546--5553},
year = 2012,
doi = {10.1021/jp3014139},
url = {http://pubs.acs.org/doi/abs/10.1021/jp3014139},
file = {::},
issn = {1932-7447},
month = {mar},
}
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