2018-04-20 08:08

5 files changed, 73 insertions, 24 deletions

diff --git a/literature/DonaldsonPaulMurray2010a.pdf b/literature/DonaldsonPaulMurray2010a.pdf
new file mode 100644
index 0000000..d65834e
--- /dev/null
+++ b/literature/DonaldsonPaulMurray2010a.pdf
diff --git a/literature/FournierFrederic2009a.pdf b/literature/FournierFrederic2009a.pdf
new file mode 100644
index 0000000..668f756
--- /dev/null
+++ b/literature/FournierFrederic2009a.pdf
diff --git a/presentation.pdf b/presentation.pdf
index cc055af..7e287ba 100644
--- a/presentation.pdf
+++ b/presentation.pdf
diff --git a/presentation.tex b/presentation.tex
index 1917763..97bd9de 100644
--- a/presentation.tex
+++ b/presentation.tex
@@ -1,7 +1,6 @@
 \documentclass{presentation}

 

-\title{Development of \\ Frequency Domain Multidimensional Spectroscopy \\

-  with Applications in Semiconductor Photophysics}

+\title{Development of \\ Frequency Domain Multidimensional Spectroscopy}

 \author{Blaise Thompson}

 

 \institute{University of Wisconsin--Madison}

@@ -14,8 +13,9 @@
 \section{CMDS}  % =================================================================================

 

 \begin{frame}{CMDS}

-	The Wright Group focuses on the development and usage of coherent multidimensional spectroscopy

-  (CMDS).

+	The Wright Group focuses on the development and usage of \\

+  Coherent MultiDimensional Spectroscopy (CMDS).

+  \vspace{\baselineskip} \\

   CMDS is a family of related nonlinear spectroscopic experiments.

 \end{frame}

    

@@ -29,16 +29,33 @@
 \end{frame}

 

 \begin{frame}{Analytical}

-  But wait! I'm an \emph{Analytical} Chemist?!

-  \\

-  The dream of the Wright Group (if not the current reality)

-  [REASONS FOR ANALYTICAL CHEMISTRY TO BE INTERESTED IN CMDS]

+  But wait! I'm an \emph{Analytical} Chemist...

+  \vspace{\baselineskip} \\

+  What am I doing in a field so rich with fundamental studies?

+  \vspace{\baselineskip} \\

+  I hope to convince you that CMDS can be used for analytical work.  % TODO: better

 \end{frame}

 

+% TODO: in fact, 2DIR is already used regularly...

+

 \begin{frame}{Analytical}  

   \fbox{\adjincludegraphics[width=\textwidth]{literature/PakoulevAndreiV2009a}}

 \end{frame}

 

+% TODO: pakoulev quotes

+

+\begin{frame}{Proteomics}

+  \fbox{\adjincludegraphics[width=\textwidth]{literature/FournierFrederic2009a}}

+\end{frame}

+

+% TODO: fournier quotes

+

+\begin{frame}{Proteomics}

+  \fbox{\adjincludegraphics[width=\textwidth]{literature/DonaldsonPaulMurray2010a}}

+\end{frame}

+

+% TODO: donaldson quotes

+  

 \section{Frequency domain}  % =====================================================================

 

 \begin{frame}{Domains of CMDS}

@@ -50,27 +67,43 @@
 \end{frame}

 

 \begin{frame}{Time domain}

-  [DESCRIPTION OF TIME DOMAIN]

+  Multiple broadband pulses are scanned in \emph{time} to collect a multidimensional interferogram.

+  \vspace{\baselineskip} \\

+  A local oscillator must be used to measure the \emph{phase} of the output.

+  \vspace{\baselineskip} \\

+  This technique is...

+  \begin{itemize}

+    \item fast (even single shot)

+    \item robust

+  \end{itemize}

+  pulse shapers have made time-domain CMDS (2DIR) almost routine.

 \end{frame}

 

 \begin{frame}{Frequency domain}

-  [DESCRIPTION OF FREQUENCY DOMAIN]

-\end{frame}

-

-\begin{frame}{Domains of CMDS}

-  Most experiments are collected in the time domain

+  In the Wright Group, we focus on \emph{frequency} domain ``Multi-Resonant'' (MR)-CMDS.

+  \vspace{\baselineskip} \\

+  Automated Optical Parametric Amplifiers (OPAs) are used to produce relatively narrow-band pulses.

+  Multidimensional spectra are collected ``directly'' by scanning OPAs against each-other.

+  \vspace{\baselineskip} \\

+  This strategy is...

   \begin{itemize}

-    \item fast

-    \item robust

+    \item slow (must directly visit each pixel)

+    \item fragile (many crucial moving pieces)

   \end{itemize}

-  So... why frequency domain?  

+  but! It is incredibly flexible.  

 \end{frame}

 

 \begin{frame}{Bandwidth}

+  MR-CMDS has no bandwidth limit!

+  \vspace{\baselineskip} \\

+  There is just the small matter of making the source continuously tunable...

   \adjincludegraphics[width=\textwidth]{opa/OPA_ranges}

 \end{frame}

 

 \begin{frame}{Selection rules}

+  MR-CMDS can easily collect data without an external local oscillator.

+  \vspace{\baselineskip} \\

+  This means... [BOYLE]

 \end{frame}

 

 \section{The instrument}  % =======================================================================

@@ -92,8 +125,10 @@
 \end{frame}

 

 \begin{frame}{Pipeline}

+  \adjincludegraphics[width=0.5\textwidth]{presentation/pipe}

   What does the ``pipeline'' of MR-CMDS data acquisition and processing look like in the Wright

-  Group? \\

+  Group?

+  \vspace{\baselineskip} \\

   How to increase data throughput and quality, while decreasing frustration of experimentalists?  %

 \end{frame}

 

@@ -101,18 +136,32 @@
 

 \begin{frame}{Processing}

   WrightTools.

-  \\

-  Universal file format.

-  \\

-  A unique, flexible multidimensional data model.

+\end{frame}

+

+\begin{frame}{Universal format}

+\end{frame}

+

+\begin{frame}{Flexible data model}

 \end{frame}

 

 \section{Acquisition}  % ==========================================================================

 

 \begin{frame}{Acquisition}

   PyCMDS.

-  \\

-  Modular software.

+\end{frame}

+

+\begin{frame}{Modular hardware model}

+\end{frame}

+

+\begin{frame}{Acquisitions}

+\end{frame}

+

+\begin{frame}{Queue}

+  This strategy can be incredibly productive!

+  \begin{itemize}

+    \item Soon after the queue was first implemented, we collected more pixels in two weeks than

+      had been collected over the previous three years.

+  \end{itemize}

 \end{frame}

 

 \section{Tuning}  % ===============================================================================

diff --git a/presentation/pipe.png b/presentation/pipe.png
new file mode 100644
index 0000000..ef81eb5
--- /dev/null
+++ b/presentation/pipe.png